Learn what "i'm not taking this anymore" means, when people say it, and how to use it naturally in English.

It means the speaker has reached their limit and will not tolerate the situation any longer.
From I Think My Wife Wants To Kill Me S2, Episode 36
Someone says they have reached their limit and will no longer accept the situation.
Use this when you want to show strong refusal to keep putting up with bad behavior or stress. It can sound angry or dramatic, so it is not polite.
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